She shuts his brunch invitation down and it's beyond cute.

Oh, what's this? The two best people in the world in one YouTube video?

Steve Buscemi is directing a Vampire Weekend webcast for American Express, whatever the hell that means, and so has been making promotional videos with the band...and now with Grimes, who is, as always, a charming beacon of charisma and perfect bangs.

Here's a video of Buscemi hanging out with Vampire Weekend, too.

ALSO PRETTY CUTE. Luv u, Buscemi, Vampire Weekend, and most of all, GRIMES.